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• W2999667083 abstract "The molecular-level structuration of two full photosystems into conjugated porous organic polymers is reported. The strategy of heterogenization gives rise to photosystems which are still fully active after 4 days of continuous illumination. Those materials catalyze the carbon dioxide photoreduction driven by visible light to produce up to three grams of formate per gram of catalyst. The covalent tethering of the two active sites into a single framework is shown to play a key role in the visible light activation of the catalyst. The unprecedented long-term efficiency arises from an optimal photoinduced electron transfer from the light harvesting moiety to the catalytic site as anticipated by quantum mechanical calculations and evidenced by in situ ultrafast time-resolved spectroscopy." @default.
• W2999667083 created "2020-01-23" @default.
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• W2999667083 date "2020-03-23" @default.
• W2999667083 modified "2023-10-16" @default.
• W2999667083 title "Molecular Porous Photosystems Tailored for Long‐Term Photocatalytic CO ₂ Reduction" @default.
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• W2999667083 doi "https://doi.org/10.1002/anie.201912883" @default.
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