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- W2999682811 abstract "A convenient strategy to enhance the aqueous stability and radiative-charge-transfer of perovskite nanocrystals (PNCs) is developed via hybriding CsPbBr3 PNCs with Ag2S nanoparticles, which is conducted by directly decomposing silver diethyldithiocarbamate in CsPbBr3 PNCs crude. The obtained CsPbBr3-Ag2S hybrids are aqueous stable, and exhibit obviously enhanced aqueous photoluminescence (PL) with a quantum yield up to 82% in pure water as well as boosted electrochemical response for charge injection and 9-fold enhanced electrochemiluminescence (ECL) than CsPbBr3 PNCs in aqueous electrolyte. Both PL and ECL spectra of CsPbBr3-Ag2S hybrids are almost identical to the PL spectrum of CsPbBr3 PNCs, indicating radiative-charge-transfer within CsPbBr3-Ag2S hybrids only occurs in CsPbBr3 segment. Annihilation ECL demonstrates that all the charges injected onto CsPbBr3-Ag2S hybrids at the redox potentials of Ag2S segment can be efficiently transferred into CsPbBr3 segment to enhance radiative-charge-transfer. This strategy is promising for the application of PNCs as well as the developing of novel electrochemiluminophores." @default.
- W2999682811 created "2020-01-23" @default.
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- W2999682811 date "2020-02-01" @default.
- W2999682811 modified "2023-10-14" @default.
- W2999682811 title "Enhanced aqueous stability and radiative-charge-transfer of CsPbBr3/Ag2S perovskite nanocrystal hybrids" @default.
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- W2999682811 doi "https://doi.org/10.1016/j.jelechem.2020.113835" @default.
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