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- W3000188821 abstract "Interfaces that can change their chemistry on demand have huge potential for applications and are prerequisites for responsive or adaptive materials. We report on the performance of a newly designed n-butyl-arylazopyrazole butyl sulfonate (butyl-AAP-C4S) surfactant that can change its structure at the air-water interface by E/Z photo-isomerization in an unprecedented way. Large and reversible changes in surface tension (Δγ = 27 mN m-1) and surface excess (ΔΓ > 2.9 μmol m-2) demonstrate superior performance of the butyl-AAP-C4S amphiphile to that of existing ionic surfactants. Neutron reflectometry and vibrational sum-frequency generation spectroscopy reveal that these large changes are caused by an unexpected monolayer-to-bilayer transition. This exceptional behavior is further shown to have dramatic consequences at larger length scales as highlighted by applications like the light-triggered collapse of aqueous foam which is tuned from high (>1 h) to low (<10 min) stabilities and light-actuated particle motion via Marangoni flows." @default.
- W3000188821 created "2020-01-23" @default.
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- W3000188821 date "2020-01-01" @default.
- W3000188821 modified "2023-09-26" @default.
- W3000188821 title "Unexpected monolayer-to-bilayer transition of arylazopyrazole surfactants facilitates superior photo-control of fluid interfaces and colloids" @default.
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- W3000188821 doi "https://doi.org/10.1039/c9sc05490a" @default.
- W3000188821 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7059314" @default.
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