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- W3000689462 abstract "Designing second-order nonlinear-optical (NLO) materials with new structures is an attractive topic. Here, a novel type of sulfide borate, Eu2B5O9S, and one of its derivatives combining S2–, I–, and borate anions in one structure (three in one), viz., Eu4.5(B5O9)2SI, are designed and synthesized with a high-temperature solid-state method. They crystallize in the noncentrosymmetric space group Pnn2. As the first sulfide borate being NLO-active, Eu4.5(B5O9)2SI demonstrates good NLO behavior, namely, a moderate powder NLO response of ca. 0.5 times and a high laser-induced damage threshold (LIDT) of ca. 15 times those of AgGaS2, and is phase-matchable. The design strategy and experimental results are verified and explained by density functional theory calculations." @default.
- W3000689462 created "2020-01-23" @default.
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- W3000689462 date "2020-01-07" @default.
- W3000689462 modified "2023-10-18" @default.
- W3000689462 title "Designing Sulfide Borate as a Novel Type of Second-Order Nonlinear-Optical Material" @default.
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- W3000689462 doi "https://doi.org/10.1021/acs.inorgchem.9b03426" @default.
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