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• W3001826931 endingPage "105696" @default.
• W3001826931 startingPage "105696" @default.
• W3001826931 abstract "Starch, as one of the most abundant, sustainable and low-cost commercial biopolymers, has versatile applications in many industries (e.g. food, paper, packaging, construction, etc.). Herein, we reported the synthesis of starch-based polyelectrolyte complexes (SPECs) barrier coatings through a straightforward, industrially scalable shear mixing process. The formation of SPECs was significantly impacted by molecular weight (MW) and charge density of starch polymer chains, resulting in SPECs with different particle sizes, particle morphologies and rheological behaviors. Larger MW and higher charge density contributed to the formation of stiff and entangled starch macromolecular network modulated by different intermolecular interactions, thus leading to a densely packed structure in the coating materials. High MW SPEC coated paperboard exhibited uniform, defect-free surface morphology, improved mechanical properties (18% and 21% increase in tensile strength and Young's modulus, respectively), and excellent barrier performance against water vapor (40% lower than uncoated paperboard), grease (Kit number of 12), and oil penetration (Cobb60: 1.85 g/m2). Such cost-effective, biodegradable and ecologically compatible SPECs barrier materials hold high potential as sustainable alternative coatings for paper and paperboard packaging applications." @default.
• W3001826931 created "2020-01-30" @default.
• W3001826931 creator A5017919922 @default.
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• W3001826931 date "2020-06-01" @default.
• W3001826931 modified "2023-10-05" @default.
• W3001826931 title "Sustainable starch-based barrier coatings for packaging applications" @default.
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• W3001826931 doi "https://doi.org/10.1016/j.foodhyd.2020.105696" @default.
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