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• W3003158785 abstract "An ordered, nanoporous polymer resin was prepared from the self-assembly of lyotropic liquid crystal monomers and employed as a heterogeneous, bifunctional catalyst. This material contains antagonistic acid and base sites in the periodic nanopores and efficiently catalyzes a model tandem reaction (i.e., the deacetalization–nitroaldol reaction between benzaldehyde dimethyl acetal and nitromethane to yield β-nitrostyrene) with excellent product selectivity. This lyotropic liquid crystal-based solid catalyst represents one of the few examples of polymeric tandem catalysts synthesized by a “bottom-up” strategy that imparts control over the stoichiometry of acidic and basic monomers and is the only reported example of a lyotropic liquid crystal-based polymer that contains mutually incompatible catalytic groups. Furthermore, this heterogeneous catalyst is highly active, exhibiting a turnover frequency for this tandem test reaction that exceeds other reported catalytic polymeric materials." @default.
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• W3003158785 date "2020-07-01" @default.
• W3003158785 modified "2023-10-14" @default.
• W3003158785 title "A nanostructured bifunctional acid–base catalyst resin formed by lyotropic liquid crystal monomers" @default.
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• W3003158785 doi "https://doi.org/10.1139/cjc-2019-0408" @default.
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