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• W3003309116 abstract "The number of developed methodologies for the ring expansion of cyclobutanol rings to five, six and seven-membered rings has increased significantly over the last six years. In this timeframe, the semipinacol rearrangement of vinyl-group containing cyclobutanols to cyclopentanones has been advanced under photoredox and electrochemical conditions, enabling the concomitant introduction of a wide array of functional groups. The expansion to 1- and 4-tetralones has been achieved for the first time under transition-metal-free conditions and even expansion to seven-membered rings has been demonstrated under rhodium catalysis. In this article, we will critically discuss the scope, application and mechanistic studies of procedures published since 2013, and provide a short outlook on the emerging potential for further development in this area." @default.
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• W3003309116 date "2020-04-01" @default.
• W3003309116 modified "2023-10-12" @default.
• W3003309116 title "Recent advances in the ring expansion of cyclobutanols, oxetanols, and azetidinols" @default.
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• W3003309116 doi "https://doi.org/10.1016/j.tetlet.2020.151695" @default.
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