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- W3004867025 abstract "A series of isostructural 3D lanthanide metal-organic frameworks (LnMOFs), with the formula n(H3O)[Ln(L)(H2O)] n ·nH2O (Ln = Gd 1, Eu 2 and Tb 3, H4L = 3,5,3',5'-oxytetrabenzoic acid), have been successfully synthesized by solvothermal reactions. Single-crystal X-ray diffraction analysis reveals that 1-3 are constructed from wave-like Ln-carboxylate chains which are further connected by the ligands to form 3D channel-type frameworks. Further experiments suggest that 3 is thermally stable up to 322 °C and exhibits outstanding chemical stability in aqueous solutions with the pH ranging from 3 to 11. Significantly, 3 can be utilized for the first time to detect malachite green (a synthetic antibiotic to cure saprolegniasis) in aqueous media even in the presence of other interfering antibiotics, with a high sensitivity (Ksv = 8.33 × 104 M-1), low detection limit (DL = 0.25 μM) and good recyclability. On a more practical note, we found that the luminescence intensity of 3 showed almost no response to pH changes (pH 3-11), allowing steady sensing in real samples such as river water, simulated human serum and urine with satisfactory recoveries and RSD." @default.
- W3004867025 created "2020-02-14" @default.
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- W3004867025 date "2020-01-01" @default.
- W3004867025 modified "2023-10-18" @default.
- W3004867025 title "A stable LnMOF as a highly efficient and selective luminescent sensor for detecting malachite green in water and real samples" @default.
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- W3004867025 doi "https://doi.org/10.1039/c9ra10870j" @default.
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