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- W3005726479 abstract "Uranium groundwater contamination due to U mining and processing affects numerous sites globally. Bioreduction of soluble, mobile U(VI) to U(IV)-bearing solids is potentially a very effective remediation strategy. Uranium isotopes (238U/235U) have been utilized to track the progress of microbial reduction, with laboratory and field studies finding a ∼1‰ isotopic fractionation, with the U(IV) product enriched in 238U. However, the isotopic fractionation produced by adsorption may complicate the use of 238U/235U to trace microbial reduction. A previous study found that adsorption of U(VI) onto Mn oxides produced a −0.2‰ fractionation with the adsorbed U(VI) depleted in 238U. In this study, adsorption to quartz, goethite, birnessite, illite, and aquifer sediments induced an average isotopic fractionation of −0.15‰ with the adsorbed U(VI) isotopically lighter than coexisting aqueous U(VI). In bicarbonate-bearing matrices, the fractionation depended little on the nature of the sorbent, with only birnessite pro..." @default.
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- W3005726479 date "2014-12-01" @default.
- W3005726479 modified "2023-09-27" @default.
- W3005726479 title "Uranium Isotopic Fractionation Induced by U(VI) Adsorption Onto Common Aquifer Minerals" @default.
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