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- W3005928381 abstract "Abstract A self-assembled coordination cage usually possesses one well-defined three-dimensional (3D) cavity whereas infinite number of 3D-cavities are crafted in a designer metal-organic framework. Construction of a discrete coordination cage possessing multiple number of 3D-cavities is a challenging task. Here we report the peripheral decoration of a trinuclear [Pd 3 L 6 ] core with one, two and three units of a [Pd 2 L 4 ] entity for the preparation of multi-3D-cavity conjoined-cages of [Pd 4 (L a ) 2 (L b ) 4 ], [Pd 5 (L b ) 4 (L c ) 2 ] and [Pd 6 (L c ) 6 ] formulations, respectively. Formation of the tetranuclear and pentanuclear complexes is attributed to the favorable integrative self-sorting of the participating components. Cage-fusion reactions and ligand-displacement-induced cage-to-cage transformation reactions are carried out using appropriately chosen ligand components and cages prepared in this work. The smaller [Pd 2 L 4 ] cavity selectively binds one unit of NO 3 − , F − , Cl − or Br − while the larger [Pd 3 L 6 ] cavity accommodates up to four DMSO molecules. Designing aspects of our conjoined-cages possess enough potential to inspire construction of exotic molecular architectures." @default.
- W3005928381 created "2020-02-24" @default.
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- W3005928381 date "2020-02-14" @default.
- W3005928381 modified "2023-10-12" @default.
- W3005928381 title "Self-assembled conjoined-cages" @default.
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- W3005928381 doi "https://doi.org/10.1038/s41467-020-14703-4" @default.
- W3005928381 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7021905" @default.
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