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• W3006422010 startingPage "1907164" @default.
• W3006422010 abstract "The methodology of metal-involved preparation for carbon materials is favored by researchers and has attracted tremendous attention. Decoupling this process and the underlying mechanism in detail are highly required. Herein, the intrinsic mechanism of carbon fixation in graphitic carbon nitride (g-C3N4) via the magnesium-involved carbonization process is reported and clarified. Magnesium can induce the displacement reaction with the small carbon nitride molecule generated by the pyrolysis of g-C3N4, thus efficiently fixing the carbon onto the in situ template of Mg3N2 product to avoid the direct volatilization. As a result, the N-doped carbon nanosheet frameworks with interconnected porous structure and suitable N content are constructed by reconstruction of carbon and nitrogen species, which exhibit a comparable photoelectric conversion efficiency (8.59%) and electrocatalytic performances to that of Pt (8.40%) for dye-sensitized solar cells." @default.
• W3006422010 created "2020-02-24" @default.
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• W3006422010 date "2020-02-16" @default.
• W3006422010 modified "2023-10-01" @default.
• W3006422010 title "Effective Fixation of Carbon in g‐C ₃ N ₄ Enabled by Mg‐Induced Selective Reconstruction" @default.
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• W3006422010 doi "https://doi.org/10.1002/smll.201907164" @default.
• W3006422010 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32064784" @default.
• W3006422010 hasPublicationYear "2020" @default.
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