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- W3007009383 abstract "• A CL instrument was developed to understand CL behavior of CO and HCs oxidation. • All the studied reactions are CL-active. • The CL method enables in-situ detection of the reaction at high sensitivity. • Good correlation between CL and reactant conversion ensures rapid screening. A chemiluminescence (CL) instrument was developed to understand the CL behavior of catalytic oxidation of CO and hydrocarbons, which are major processes occurring in catalytic converters. The instrument is based on the cooperation among a gas mixer, a custom-made CL analyzer, and an on-line gas chromatography. The concept of the CL method was formulated by thoroughly investigating the CL emission during the catalytic oxidation of CO and C 3 H 6 in the presence of O 2 and/or NO under both stoichiometric and non-stoichiometric conditions. All the oxidation reactions were found to be CL-active, where the CL intensity increased exponentially with the temperature. The steady-state measurements showed good linearity between the CL intensity and the reaction rates, demonstrating that the CL emission is a direct product of the reactions. It was also found that the CL intensity per CO 2 production was different among the reactions, most plausibly due to both/either the presence of multiple CL processes and/or the difference in the heat of the reactions. Based on the linear correlation between the CL intensity and the reaction rate, a feasibility study was successfully demonstrated for rapid catalyst evaluation in C 3 H 6 oxidation." @default.
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- W3007009383 date "2021-09-01" @default.
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- W3007009383 title "Understanding chemiluminescence in catalytic oxidation of CO and hydrocarbons" @default.
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- W3007009383 doi "https://doi.org/10.1016/j.cattod.2020.02.034" @default.
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