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- W3007517618 abstract "Abstract Extension and clustering of polycyclic aromatic hydrocarbons (PAHs) are key mechanistic steps for coking and deactivation in catalysis reactions. However, no unambiguous mechanistic picture exists on molecule-resolved PAHs speciation and evolution, due to the immense experimental challenges in deciphering the complex PAHs structures. Herein, we report an effective strategy through integrating a high resolution MALDI FT-ICR mass spectrometry with isotope labeling technique. With this strategy, a complete route for aromatic hydrocarbon evolution is unveiled for SAPO-34-catalyzed, industrially relevant methanol-to-olefins (MTO) as a model reaction. Notable is the elucidation of an unusual, previously unrecognized mechanistic step: cage-passing growth forming cross-linked multi-core PAHs with graphene-like structure. This mechanistic concept proves general on other cage-based molecule sieves. This preliminary work would provide a versatile means to decipher the key mechanistic step of molecular mass growth for PAHs involved in catalysis and combustion chemistry." @default.
- W3007517618 created "2020-03-06" @default.
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- W3007517618 date "2020-02-26" @default.
- W3007517618 modified "2023-10-16" @default.
- W3007517618 title "Molecular elucidating of an unusual growth mechanism for polycyclic aromatic hydrocarbons in confined space" @default.
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- W3007517618 doi "https://doi.org/10.1038/s41467-020-14493-9" @default.
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