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- W3008488961 abstract "By a selective three‐component multi‐catalytic sequence, amino‐catalyzed oxa‐Michael addition of oximes to α,β‐unsaturated aldehydes has been combined with a copper‐catalyzed decarboxylative aldolization. This one‐pot procedure enables the rapid construction of functionalized ketodiol scaffolds in 85 to 94% ee . Simple reduction of both the resulting oxime and ketone functions delivered the corresponding 1,3,5‐triols of interest in a minimum of steps while considerably limiting waste generation. This methodology has been applied to the shortest (4 steps) synthesis of (+)‐yashabushitriol, highlighting the synthetic potential of this new multi‐catalytic sequence." @default.
- W3008488961 created "2020-03-06" @default.
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- W3008488961 date "2020-03-05" @default.
- W3008488961 modified "2023-10-16" @default.
- W3008488961 title "Three-Component Multi-Catalytic Enantioselective Oxa-Michael/Aldolization Sequence and Application to (+)-Yashabushitriol Synthesis" @default.
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- W3008488961 doi "https://doi.org/10.1002/ejoc.202000185" @default.
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