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- W3008577041 abstract "CO2 and H2O can be energy-upgraded through solar thermochemical cycles. Suitable redox materials are reduced in a solar reactor at high temperature (above 1300-1400°C) and afterwards re-oxidised by CO2 and/or H2O flow, thus producing CO and/or H2. Ceria was recognised as one of the most interesting materials for this process. However, high reduction temperature, low re-oxidation kinetics as well as low stability hindered its practical application. In this work, the redox properties of Ce0.75Zr0.25O2 system prepared by hydrothermal synthesis were compared with those of a co-precipitated sample with the same nominal composition used as reference. Samples were characterised by XRD and N2 physisorption; their self-reducibility and CO2 splitting activity were tested in a thermogravimetric balance, while H2O splitting properties were studied in an ad hoc fixed bed reactor on H2 pre-reduced samples. Obtained results proved that the material prepared by hydrothermal synthesis is characterised by both improved reducibility and splitting activity." @default.
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- W3008577041 date "2019-05-31" @default.
- W3008577041 modified "2023-09-23" @default.
- W3008577041 title "Syngas Production Through H2o/co2 Thermochemical Splitting" @default.
- W3008577041 doi "https://doi.org/10.3303/cet1974008" @default.
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