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• W3009028462 startingPage "6103" @default.
• W3009028462 abstract "This study has shown that the electrocatalytic activity of gold nanoparticles (Au NPs) is the key factor governing the performance of Au NP-loaded TiO2 plasmonic electrodes for the water oxidation reaction. Au NPs were loaded onto the mesoporous rutile TiO2 nanocrystalline film (Au/mp-TiO2) and rutile TiO2 nanowire array (Au/TiO2-NWA) electrodes by the deposition–precipitation method. Faceted Au NPs with sharp edges and corners are formed on TiO2-NWA, while the Au NPs on mp-TiO2 are almost non-faceted and hemisphere-like. An ultrathin Cu shell layer was formed selectively on the Au surface of Au/TiO2-NWA to yield Au(core)–Cu(shell) NPs on TiO2-NWA (Au@Cu/TiO2-NWA) by the photodeposition technique. Electrochemical measurements showed that the electrocatalytic activity of the water oxidation reaction significantly depends on the shape of Au NPs and Cu shell formation, and their order of dependence is Au/mp-TiO2 < Au/TiO2-NWA < Au@Cu/TiO2-NWA. Furthermore, the action spectra of incident photon-to-current conversion efficiency indicated that the increase in the electrocatalytic activity enhances the photocurrent at a given excitation wavelength, simultaneously extending the spectral response range." @default.
• W3009028462 created "2020-03-06" @default.
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• W3009028462 date "2020-02-24" @default.
• W3009028462 modified "2023-09-24" @default.
• W3009028462 title "Electrocatalytic Effect on the Photon-to-Current Conversion Efficiency of Gold-Nanoparticle-Loaded Titanium(IV) Oxide Plasmonic Electrodes for Water Oxidation" @default.
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• W3009028462 doi "https://doi.org/10.1021/acs.jpcc.9b11207" @default.
• W3009028462 hasPublicationYear "2020" @default.
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