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• W3009325339 abstract "Anactivated carbon-supported Cu/ZnO catalyst for CO2 hydrogenationto methanol has been prepared by the facile plasmadecomposition of a Cu–Zn precursor at moderate temperature.The Cu/ZnO/C catalyst prepared by cold plasma featured smaller sizeand higher dispersion than that prepared by traditional calcination.The low operation temperature plays an important role in this. Thecatalysts are characterized using a multitechnique approach. X-rayphotoelectron spectroscopy results indicate that cold plasma can introducespecific O-containing groups on the carbon surface. It also facilitatesthe dispersion of active components and H spillover. H2 temperature-programmed reduction profiles and transmission electronmicroscopy images show that the interaction between Cu, ZnO, and carbonin the Cu/ZnO/C catalyst prepared by cold plasma was stronger thanthat in the catalyst prepared by calcination. The properties are beneficialto the CO2 hydrogenation reaction. The catalytic performanceof the catalysts was tested in a fixed-bed reactor. The Cu/ZnO/C catalystprepared by cold plasma showed an obvious increase in CO2 conversion, methanol selectivity, and productivity in the catalyticevaluation of catalysts. Moreover, it obtained a remarkable space-timeyield of 92.5 gmethanol·kgcat–1·h–1 at 260 °C that is approximately1.5 times that of Cu/ZnO/C prepared by calcination." @default.
• W3009325339 created "2020-03-13" @default.
• W3009325339 creator A5036854394 @default.
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• W3009325339 date "2020-03-02" @default.
• W3009325339 modified "2023-09-27" @default.
• W3009325339 title "Enhanced Activity of Cu/ZnO/C Catalysts Prepared by Cold Plasma for CO₂ Hydrogenation to Methanol" @default.
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• W3009325339 doi "https://doi.org/10.1021/acs.iecr.9b06996" @default.
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