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• W3009467309 abstract "Abstract Isotopic ratios of radioactive releases into the environment are useful signatures for contamination source assessment. Uranium is known to behave conservatively in sea water so that a ratio of uranium trace isotopes may serve as a superior oceanographic tracer. Here we present data on the atomic $$^{233}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>233</mml:mn></mml:mrow></mml:msup></mml:math> U/ $$^{236}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>236</mml:mn></mml:mrow></mml:msup></mml:math> U ratio analyzed in representative environmental samples finding ratios of (0.1–3.7) $$cdot$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mo>⋅</mml:mo></mml:math> 10 $$^{-2}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mo>−</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:math> . The ratios detected in compartments of the environment affected by releases of nuclear power production or by weapons fallout differ by one order of magnitude. Significant amounts of $$^{233}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>233</mml:mn></mml:mrow></mml:msup></mml:math> U were only released in nuclear weapons fallout, either produced by fast neutron reactions or directly by $$^{233}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>233</mml:mn></mml:mrow></mml:msup></mml:math> U-fueled devices. This makes the $$^{233}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>233</mml:mn></mml:mrow></mml:msup></mml:math> U/ $$^{236}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>236</mml:mn></mml:mrow></mml:msup></mml:math> U ratio a promising new fingerprint for radioactive emissions. Our findings indicate a higher release of $$^{233}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow /><mml:mrow><mml:mn>233</mml:mn></mml:mrow></mml:msup></mml:math> U by nuclear weapons tests before the maximum of global fallout in 1963, setting constraints on the design of the nuclear weapons employed." @default.
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• W3009467309 date "2020-03-09" @default.
• W3009467309 modified "2023-10-14" @default.
• W3009467309 title "233U/236U signature allows to distinguish environmental emissions of civil nuclear industry from weapons fallout" @default.
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• W3009467309 doi "https://doi.org/10.1038/s41467-020-15008-2" @default.
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