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- W3010037801 abstract "Abstract Hierarchical porous g-C3N4 nanosheets are prepared from melamine using NH4Cl as dynamic gas templates to anchor the ultrafine Ru nanoparticles (NPs) with a facile adsorption-in situ reduction strategy. The results reveal that 1: 3 is the optimal mass ratio for melamine to NH4Cl and the Ru NPs are evenly dispersed in the porous network of g-C3N4 in the corresponding catalysts. Remarkably, the porous catalysts exhibit superior catalytic activity and satisfactory recyclability for ammonia borane (NH3-BH3, AB) hydrolysis. The corresponding turnover frequency is as high as 122.2 × 103 mL H 2 · g Ru -1 · min -1 and the apparent activation energy (35.6 kJ mol−1) is competitive. AB hydrolysis is of 1.17-order and near zero-order with respect to the Ru and AB concentrations, respectively. The results demonstrate that the Ru/g-C3N4 catalysts are promising in developing an alternative clean and environmentally friendly energy carrier from the hydrogen storage materials." @default.
- W3010037801 created "2020-03-13" @default.
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- W3010037801 date "2020-04-01" @default.
- W3010037801 modified "2023-09-23" @default.
- W3010037801 title "Ultrafine Ru nanoparticles anchored to porous g-C3N4 as efficient catalysts for ammonia borane hydrolysis" @default.
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- W3010037801 doi "https://doi.org/10.1016/j.apcata.2020.117511" @default.
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