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- W3010343500 abstract "Abstract We first studied the reactivity of H 2 O vapor in metal–organic frameworks (MOFs) with Pt nanocrystals (NCs) through the water–gas shift (WGS) reaction. A water‐stable MOF, UiO‐66, serves as a highly effective support material for the WGS reaction compared with ZrO 2 . The origin of the high catalytic performance was investigated using in situ IR spectroscopy. In addition, from a comparison of the catalytic activities of Pt on UiO‐66, where Pt NCs are located on the surface of UiO‐66 and Pt@UiO‐66, where Pt NCs are coated with UiO‐66, we found that the competitive effects of H 2 O condensation and diffusion in the UiO‐66 play important roles in the catalytic activity of Pt NCs. A thinner UiO‐66 coating further enhanced the WGS reaction activity of Pt NCs by minimizing the negative effect of slow H 2 O diffusion in UiO‐66." @default.
- W3010343500 created "2020-03-13" @default.
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- W3010343500 date "2019-07-22" @default.
- W3010343500 modified "2023-09-27" @default.
- W3010343500 title "The First Study on the Reactivity of Water Vapor in Metal–Organic Frameworks with Platinum Nanocrystals" @default.
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- W3010343500 doi "https://doi.org/10.1002/anie.201905667" @default.
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