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• W3010924105 startingPage "110172" @default.
• W3010924105 abstract "Large crystals of silicalite (0.1–1 mm) were synthesized and used to study the kinetics and equilibrium of CO2 adsorption (at room temperature), both as a pure component and as a binary mixture with nitrogen, using Infra-Red Microscopy (IRM) coupled with Fourier Transform Infra-Red Spectroscopy (FTIR). The use of such large crystals permits the measurement of fast intra-crystalline diffusion processes, beyond the range normally accessible by macroscopic techniques. As expected the effect of N2 on the CO2 equilibrium was minimal but the effect on the intra-crystalline diffusivity was significant. Diffusivities (at 300 K) range from 4 × 10−8 to 4 × 10−9 m2 s−1 for CO2, decreasing with increasing total concentrations of CO2 and N2 in the adsorbed phase." @default.
• W3010924105 created "2020-03-23" @default.
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• W3010924105 date "2020-06-01" @default.
• W3010924105 modified "2023-09-27" @default.
• W3010924105 title "Equilibrium isotherms and transport diffusivities for CO2 and CO2/N2 mixtures in silicalite measured by Infra-Red Micro-imaging" @default.
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• W3010924105 doi "https://doi.org/10.1016/j.micromeso.2020.110172" @default.
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