Matches in SemOpenAlex for { <https://semopenalex.org/work/W3011101236> ?p ?o ?g. }
- W3011101236 endingPage "17527" @default.
- W3011101236 startingPage "17519" @default.
- W3011101236 abstract "Hydrogen peroxide (H2O2) production by electrocatalytic two-electron oxygen reduction shows promise as a replacement for energy-intensive anthraquinone oxidation or H2/O2 direct synthesis. Here, we report on graphene-supported Ni single-atom (SA) electrocatalysts, which are synthesized by a simple surfactant-free reduction process with enhanced electrocatalytic activity and stability. Unlike conventional Ni nanoparticles or alloy catalysts, the well-dispersed Ni-SA sites lack adjacent Ni atoms. This structure promotes H2O2 production by a two-electron oxygen reduction pathway under an alkaline condition (pH = 13). This catalyst exhibited enhanced H2O2 selectivity (>94%) with a considerable mass activity (2.11 A mgNi-1 at 0.60 V vs reversible hydrogen electrode), owing to the presence of oxygen functional groups and isolated Ni sites. Density functional theory calculations provide insights into the role of this catalyst in optimizing the two-electron oxygen reduction reaction pathway with high H2O2 selectivity. This work suggests a new method for controlling reaction pathways in atomically dispersed non-noble catalysts." @default.
- W3011101236 created "2020-03-23" @default.
- W3011101236 creator A5006960816 @default.
- W3011101236 creator A5012278873 @default.
- W3011101236 creator A5031810848 @default.
- W3011101236 creator A5054564234 @default.
- W3011101236 creator A5073152857 @default.
- W3011101236 creator A5086471424 @default.
- W3011101236 creator A5090366405 @default.
- W3011101236 creator A5091588180 @default.
- W3011101236 date "2020-03-20" @default.
- W3011101236 modified "2023-10-16" @default.
- W3011101236 title "Graphene-Supported Single Nickel Atom Catalyst for Highly Selective and Efficient Hydrogen Peroxide Production" @default.
- W3011101236 cites W1753266278 @default.
- W3011101236 cites W1972243282 @default.
- W3011101236 cites W1979544533 @default.
- W3011101236 cites W1981368803 @default.
- W3011101236 cites W1982153238 @default.
- W3011101236 cites W1994211019 @default.
- W3011101236 cites W2032819879 @default.
- W3011101236 cites W2033342187 @default.
- W3011101236 cites W2039527261 @default.
- W3011101236 cites W2044591029 @default.
- W3011101236 cites W2061367556 @default.
- W3011101236 cites W2070227796 @default.
- W3011101236 cites W2080475618 @default.
- W3011101236 cites W2083222334 @default.
- W3011101236 cites W2087207644 @default.
- W3011101236 cites W2110534188 @default.
- W3011101236 cites W2114291507 @default.
- W3011101236 cites W2118708336 @default.
- W3011101236 cites W2131475384 @default.
- W3011101236 cites W2133170178 @default.
- W3011101236 cites W2160174308 @default.
- W3011101236 cites W2167035995 @default.
- W3011101236 cites W2197330948 @default.
- W3011101236 cites W2221132146 @default.
- W3011101236 cites W2262245919 @default.
- W3011101236 cites W2297872481 @default.
- W3011101236 cites W2315546872 @default.
- W3011101236 cites W2336039729 @default.
- W3011101236 cites W2491138686 @default.
- W3011101236 cites W2502288548 @default.
- W3011101236 cites W2531629454 @default.
- W3011101236 cites W2536987324 @default.
- W3011101236 cites W2550231030 @default.
- W3011101236 cites W2550657007 @default.
- W3011101236 cites W2554421598 @default.
- W3011101236 cites W2564196652 @default.
- W3011101236 cites W2606430471 @default.
- W3011101236 cites W2617194355 @default.
- W3011101236 cites W2625660734 @default.
- W3011101236 cites W2756103432 @default.
- W3011101236 cites W2758351518 @default.
- W3011101236 cites W2782723324 @default.
- W3011101236 cites W2783420615 @default.
- W3011101236 cites W2785768358 @default.
- W3011101236 cites W2795272585 @default.
- W3011101236 cites W2795293472 @default.
- W3011101236 cites W2801820474 @default.
- W3011101236 cites W2805483123 @default.
- W3011101236 cites W2806106740 @default.
- W3011101236 cites W2809925599 @default.
- W3011101236 cites W2865912219 @default.
- W3011101236 cites W2889210469 @default.
- W3011101236 cites W2891982331 @default.
- W3011101236 cites W2900604663 @default.
- W3011101236 cites W2971471509 @default.
- W3011101236 doi "https://doi.org/10.1021/acsami.0c01278" @default.
- W3011101236 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32195568" @default.
- W3011101236 hasPublicationYear "2020" @default.
- W3011101236 type Work @default.
- W3011101236 sameAs 3011101236 @default.
- W3011101236 citedByCount "90" @default.
- W3011101236 countsByYear W30111012362020 @default.
- W3011101236 countsByYear W30111012362021 @default.
- W3011101236 countsByYear W30111012362022 @default.
- W3011101236 countsByYear W30111012362023 @default.
- W3011101236 crossrefType "journal-article" @default.
- W3011101236 hasAuthorship W3011101236A5006960816 @default.
- W3011101236 hasAuthorship W3011101236A5012278873 @default.
- W3011101236 hasAuthorship W3011101236A5031810848 @default.
- W3011101236 hasAuthorship W3011101236A5054564234 @default.
- W3011101236 hasAuthorship W3011101236A5073152857 @default.
- W3011101236 hasAuthorship W3011101236A5086471424 @default.
- W3011101236 hasAuthorship W3011101236A5090366405 @default.
- W3011101236 hasAuthorship W3011101236A5091588180 @default.
- W3011101236 hasConcept C118792377 @default.
- W3011101236 hasConcept C123480859 @default.
- W3011101236 hasConcept C127413603 @default.
- W3011101236 hasConcept C147789679 @default.
- W3011101236 hasConcept C161790260 @default.
- W3011101236 hasConcept C171250308 @default.
- W3011101236 hasConcept C17525397 @default.
- W3011101236 hasConcept C178790620 @default.
- W3011101236 hasConcept C179104552 @default.
- W3011101236 hasConcept C185592680 @default.
- W3011101236 hasConcept C191897082 @default.