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• W3011639046 abstract "Abstract Although polymers have been studied for well over a century, there are few examples of covalently linked polymer crystals synthesised directly from solution. One-dimensional (1D) covalent polymers that are packed into a framework structure can be viewed as a 1D covalent organic framework (COF), but making a single crystal of this has been elusive. Herein, by combining labile metal coordination and dynamic covalent chemistry, we discover a strategy to synthesise single-crystal metallo-COFs under solvothermal conditions. The single-crystal structure is rigorously solved using single-crystal electron diffraction technique. The non-centrosymmetric metallo-COF allows second harmonic generation. Due to the presence of syntactic pendant amine groups along the polymer chains, the metallopolymer crystal can be further cross-linked into a crystalline woven network." @default.
• W3011639046 created "2020-03-23" @default.
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• W3011639046 date "2020-03-18" @default.
• W3011639046 modified "2023-10-05" @default.
• W3011639046 title "Single crystal of a one-dimensional metallo-covalent organic framework" @default.
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• W3011639046 doi "https://doi.org/10.1038/s41467-020-15281-1" @default.
• W3011639046 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7080745" @default.
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• W3011639046 hasPublicationYear "2020" @default.
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