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- W3012084564 abstract "Direct formic acid fuel cells have great application potential in the energy field, but their commercialization is hindered by the CO poisoning and low performance of Pd-based anode catalysts. In this study, novel composite catalysts composed of Pd, organic-inorganic hybrid imidazole ionic liquid polyoxometalates, and N,P-codoped coal-based carbon fibers with good dispersion and smaller Pd nanoparticles were synthesized successfully. Physical and electrochemical characterizations revealed that the as-prepared Pd-based composite catalysts have excellent CO poisoning resistance and enhanced electrocatalytic activity in formic acid electrooxidation. Notably, the CO oxidation onset potential of a catalyst modified by imidazole ionic liquid polyoxometalate with long alkyl chain was 0.1 V lower than that of the unmodified catalyst. The mass activity of the as-prepared Pd catalyst in formic acid oxidation was 754.1 mA mg−1Pd. It is expected that organic-inorganic hybrid polyoxometalates can be further applied to fuel cell catalysts." @default.
- W3012084564 created "2020-03-23" @default.
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- W3012084564 date "2020-06-01" @default.
- W3012084564 modified "2023-10-17" @default.
- W3012084564 title "Ionic liquid polyoxometalate-enhanced Pd/N,P-codoped coal-based carbon fiber catalysts for formic acid electrooxidation" @default.
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- W3012084564 doi "https://doi.org/10.1016/j.apsusc.2020.146137" @default.
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