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- W3012090390 abstract "A pomegranate-like cathode, VN/[email protected], is synthesized according to a simple principle of electrostatic attraction through a controllable Zeta potential method, establishing a hierarchical-structured VN/S nanoclusters encapsuled with graphene nanosheets. Internal VN nanoparticles trap lithium polysulphides (LiPSs) and catalyse them transforming from long-chain to short-chain species; whereas the external cladding layers of graphene nanosheets confine the transformations in a nanoscale-catalysis reactors. VN/[email protected] cathode exhibits excellent long-cycling life at 2 C rate during the 2000 cycles, corresponding to 0.038 percent of capacity fade per cycle. According to in-situ Raman and electrochemical impedance spectroscopies, VN catalyst accelerates chemical transformations of liquid-state LiPSs to solid-state Li2S2/Li2S and graphene intensifies Li+ diffusion behaviour. Improvement of electrochemical performance of the VN/[email protected] cathode depends on a coefficient of physical and chemical interactions between VN catalyst and LiPSs species." @default.
- W3012090390 created "2020-03-23" @default.
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- W3012090390 date "2020-04-01" @default.
- W3012090390 modified "2023-09-26" @default.
- W3012090390 title "VN/S Nanoclusters Encapsulated with Graphene via Zeta Potential Control: A Pomegranate‐Like Cathode for Lithium‐Sulfur Batteries with Enhanced Rate Performance" @default.
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- W3012090390 doi "https://doi.org/10.1002/celc.202000163" @default.
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