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• W3012199568 abstract "A series of luminescent aryloxy-benzothiadiazole derivatives with architectures ArO-BTD-Ar’ and ArO-BTD-NAr’ were synthetized. The aim was to achieve a molecular design based on restriction of intramolecular rotation of the ArO- group associated to the presence of bulky aryl or N -aryl groups, which can avoid detrimental π-π stacking and favor radiative decays in the aggregated/solid state. In solution, these compounds showed fluorescence emission located in the blue to red regions with relative high fluorescence quantum yields (φ FL = 0.27–0.74). For all ArO-BTD-Ar’ derivatives, emission enhancement was observed upon aggregation. The essential role of the ArO- group in the AIEEgenic ability was confirmed by comparing with Ar’-BTD-Ar’ analogs. Some solid ArO-BTD-Ar’ compounds displayed higher φ FL than when in solution. Their aggregation-induced enhanced emission (AIEE) were corroborated by studies in water/acetone systems (I/I 0 emission rations up to 7.7). Monocrystal X-ray analysis of selected compounds confirmed the twisted nature and absence of detrimental π-π stacking. The more emissive compound (φ FL = 0.83) was applied as emitting material in a green OLED structure, presenting turn-on voltage around 3.5 V and luminance up to 1200 cd m −2 , with a maximum current efficiency of 5.6 × 10 −1 cd A −1 at 6.5 V. • Aryloxy-BTD derivatives were designed aiming AIEE. • Blue to red fluorescence emission with φ FL = 0.27–0.74 were observed in solution. • Some solid ArO-BTD-Ar’ compounds display higher φ FL than when in solution. • All ArO-BTD-Ar’ derivatives show AIEE (I/I 0 up to 7.7). • The more emissive solid compound (φ FL = 0.83) was applied as emitter in a OLED." @default.
• W3012199568 created "2020-03-23" @default.
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• W3012199568 date "2020-07-01" @default.
• W3012199568 modified "2023-09-26" @default.
• W3012199568 title "Designing highly luminescent aryloxy-benzothiadiazole derivatives with aggregation-induced enhanced emission" @default.
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• W3012199568 doi "https://doi.org/10.1016/j.dyepig.2020.108377" @default.
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