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• W3012334196 endingPage "17805" @default.
• W3012334196 startingPage "17799" @default.
• W3012334196 abstract "Poly(3,4-ethylenedioxythiophene):poly(4-styrene sulfonate) (PEDOT:PSS) has demonstrated outstanding performance as a charge transport layer or an electrode in various electronic devices, including organic solar cells, organic light-emitting diodes, and organic field-effect transistors (OFETs). The electrical properties of these devices are affected by the contact properties at the PEDOT:PSS–semiconductor junction. In this research, we performed work function (WF) engineering of electrohydrodynamic (EHD)-jet-printed PEDOT:PSS and successfully used it as an electrode to fabricate high-performance OFETs and complementary logic circuits. Two types of PEDOT:PSS materials–one with a high WF (HWF, 5.28 eV) and the other with a low WF (LWF, 4.53 eV)–were synthesized and EHD-jet-printed. The WF of PEDOT:PSS was deterministically modulated by approximately 0.75 eV through simple mixing of the two synthesized PEDOT:PSS materials in various ratios. OFETs fabricated with HWF and LWF PEDOT:PSS electrodes showed excellent electrical properties, including the ON/OFF switching ratio higher than 107 and the highest carrier mobility greater than 1 cm2·V–1·s–1. Furthermore, the HWF and LWF PEDOT:PSS electrodes were integrated to fabricate complementary metal–oxide–semiconductor (CMOS) NOT, NOR, and NAND circuits." @default.
• W3012334196 created "2020-03-23" @default.
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• W3012334196 date "2020-03-18" @default.
• W3012334196 modified "2023-10-11" @default.
• W3012334196 title "Work Function Engineering of Electrohydrodynamic-Jet-Printed PEDOT:PSS Electrodes for High-Performance Printed Electronics" @default.
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• W3012334196 doi "https://doi.org/10.1021/acsami.0c02580" @default.
• W3012334196 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32186179" @default.
• W3012334196 hasPublicationYear "2020" @default.
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