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- W3012654573 abstract "Abstract Capillary condensation within the pore space formed by a hexagonal arrangement of carbon nanorods is investigated using a thermodynamic model. Numerical solution of the corresponding non-linear differential equations predicts two characteristic equilibrium phase transitions corresponding to liquid-bridge formation between adjacent rods, and the subsequent filling of the entire pore space with liquid adsorbate at higher relative pressure, respectively. These separate transitions are predicted for a wide range of porosities, as demonstrated for two non-polar fluids, nitrogen and n-pentane, employing experimentally determined reference isotherms to model the fluid–solid interactions. The theoretical predictions are compared to experimental data for nitrogen and n-pentane adsorption in an ordered mesoporous CMK-3 type material, with the necessary structural parameters obtained from small-angle X-ray scattering. Although the experimental adsorption isotherms do not unambiguously show two separate transitions due to a high degree of structural disorder of the mesopore space, their general trends are consistent with the theoretical predictions for both adsorbates." @default.
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- W3012654573 date "2020-03-21" @default.
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- W3012654573 title "Capillary bridge formation between hexagonally ordered carbon nanorods" @default.
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- W3012654573 doi "https://doi.org/10.1007/s10450-020-00215-6" @default.
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