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- W3012806242 abstract "Metal–nitrogen–carbon (MNC) nanocomposites have been hailed as promising and efficient electrocatalysts toward oxygen reduction reaction (ORR), due to the formation of MNx coordination moieties. However, MNC hybrids are mostly prepared by pyrolysis of organic precursors along with select metal salts, where part of the MNx sites are inevitably buried in the carbon matrix. This limited accessibility compromises the electrocatalytic performance. Herein, we describe a wet-impregnation procedure by facile thermal refluxing, whereby palladium is atomically dispersed and enriched onto the surface of hollow, nitrogen-doped carbon cages (HNC) forming Pd–N coordination bonds. The obtained Pd-HNC nanocomposites exhibit an ORR activity in alkaline media markedly higher than that of metallic Pd nanoparticles, and the best sample even outperforms commercial Pt/C and relevant Pd-based catalysts reported in the literature. The results suggest that atomic dispersion and surface enrichment of palladium in a carbon matrix may serve as an effective strategy in the fabrication of high-performance ORR electrocatalysts." @default.
- W3012806242 created "2020-03-27" @default.
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- W3012806242 date "2020-03-23" @default.
- W3012806242 modified "2023-10-04" @default.
- W3012806242 title "Atomic Dispersion and Surface Enrichment of Palladium in Nitrogen-Doped Porous Carbon Cages Lead to High-Performance Electrocatalytic Reduction of Oxygen" @default.
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- W3012806242 cites W1980929676 @default.
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- W3012806242 cites W2022299938 @default.
- W3012806242 cites W2022888795 @default.
- W3012806242 cites W2023967155 @default.
- W3012806242 cites W2025611237 @default.
- W3012806242 cites W2032570058 @default.
- W3012806242 cites W2032691156 @default.
- W3012806242 cites W2063313108 @default.
- W3012806242 cites W2070227796 @default.
- W3012806242 cites W2073872893 @default.
- W3012806242 cites W2088224528 @default.
- W3012806242 cites W2161685244 @default.
- W3012806242 cites W2167035995 @default.
- W3012806242 cites W2227368397 @default.
- W3012806242 cites W2235279340 @default.
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- W3012806242 cites W2418439740 @default.
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- W3012806242 cites W2564518721 @default.
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- W3012806242 doi "https://doi.org/10.1021/acsami.0c03415" @default.
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- W3012806242 hasPublicationYear "2020" @default.
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