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- W3013037080 abstract "Abstract Most synthetic building blocks self‐assemble into one‐ or three‐dimensional architectures. However, fewer examples have been reported on the aggregation of amphiphiles to form optically‐active two‐dimensional (2D) structures. Herein, we report the self‐assembly of tetraphenylethylene (TPE)‐containing hydrophilic dendrons into 2D sheet structures in aqueous methanol solution. TEM and AFM investigations showed that the self‐assembly of disubstituted TPE generates helical nanofibers as an intermediate structure which, in turn, laterally associate into a chiral sheet structure with a thickness of 4.6 nm, whereas tetrasubstituted TPE self‐assembles into a nonchiral sheet structure with a thickness of 3.8 nm. In great contrast to the nonchiral sheets, the chiral sheets are able to preferentially absorb the d ‐enantiomer in a racemic phenylalanine derivative solution accompanied by fluorescence enhancement, thus indicating that the single‐layered chiral sheets act as an enantioselective membrane that can be used for fluorescence sensing." @default.
- W3013037080 created "2020-04-03" @default.
- W3013037080 creator A5029732076 @default.
- W3013037080 creator A5037862752 @default.
- W3013037080 date "2020-04-01" @default.
- W3013037080 modified "2023-10-10" @default.
- W3013037080 title "Self‐Assembly of Tetraphenylethylene‐Based Amphiphiles in Aqueous Methanol Solution into Two‐Dimensional Chiral Sheets for Enantioselective Sorption" @default.
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- W3013037080 doi "https://doi.org/10.1002/cplu.202000130" @default.
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