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• W3013058293 abstract "Abstract The photocatalytic activity of P25 TiO 2 with 0.36 % (w/w) Pt co‐catalyst towards the formation of methane, in the presence of CO 2 and H 2 O vapor, is investigated in a flow photoreactor under varying reaction conditions of temperature, water molar fraction in the dosed gas and residence time. Within the range of parameters studied, H 2 O molar fraction is found to be the most sensitive parameter, and its increase leads to larger production rates as well as to a significant slow down of photocatalytic activity loss. This observed activation with water content is in contrast to the effect known in neat P25 and it occurs in a regime of very large adsorbed H 2 O to CO 2 excess, and can be understood in the context of hole extraction being much slower than electron extraction. These results also constrain the possible interpretation of the nature of the photocatalyst deactivation processes." @default.
• W3013058293 created "2020-04-03" @default.
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• W3013058293 date "2020-04-23" @default.
• W3013058293 modified "2023-09-27" @default.
• W3013058293 title "Investigation of reaction condition effects on photocatalytic methane production over P25‐TiO ₂ /Pt with CO ₂ and H ₂ O gas. Applied and mechanistic implications" @default.
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• W3013058293 doi "https://doi.org/10.1002/cptc.202000018" @default.
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