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- W3013225966 abstract "We report the catalytic asymmetric synthesis of Tafluprost (1), a prostaglandin analogue. This synthesis demonstrates a new approach to prostaglandins involving symmetrization and desymmetrization of a racemic precursor to control the absolute and relative stereochemistry of the cyclopentyl core. Key steps include a diastereo- and enantioselective Rh-catalyzed Suzuki–Miyaura reaction of a racemic bicyclic allyl chloride and an alkenyl boronic acid and a regio- and diastereoselective Pd-catalyzed Tsuji–Trost reaction with an enolate surrogate." @default.
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- W3013225966 date "2020-03-27" @default.
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- W3013225966 title "An Asymmetric Suzuki–Miyaura Approach to Prostaglandins: Synthesis of Tafluprost" @default.
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- W3013225966 doi "https://doi.org/10.1021/acs.orglett.0c00745" @default.
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