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• W3014149124 abstract "It has been technically challenging to concurrently probe the electrons and the lattices in materials during nonequilibrium processes, allowing their correlations to be determined. Here, in a single set of ultrafast electron diffraction patterns taken on the charge-density-wave (CDW) material $1T$-TaSeTe, we discover a temporal shift in the diffraction intensity measurements as a function of scattering angle. With the help of dynamic models and theoretical calculations, we show that the ultrafast electrons probe both the valence-electron and lattice dynamic processes, resulting in the temporal shift measurements. Our results demonstrate unambiguously that the CDW is not merely a result of the periodic lattice deformation ever present in $1T$-TaSeTe but has significant electronic origin. This method demonstrates an approach for studying many quantum effects that arise from electron-lattice dephasing in molecules and crystals for next-generation devices." @default.
• W3014149124 created "2020-04-10" @default.
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• W3014149124 date "2020-03-31" @default.
• W3014149124 modified "2023-10-15" @default.
• W3014149124 title "Concurrent probing of electron-lattice dephasing induced by photoexcitation in <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:mn>1</mml:mn><mml:mi>T</mml:mi></mml:mrow></mml:math> -TaSeTe using ultrafast electron diffraction" @default.
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• W3014149124 doi "https://doi.org/10.1103/physrevb.101.100304" @default.
• W3014149124 hasPublicationYear "2020" @default.
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