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• W3014320178 endingPage "118309" @default.
• W3014320178 startingPage "118309" @default.
• W3014320178 abstract "The photophysical properties of iridium(III) porphyrins complexes with two different axial ligands (Cl(CO) and bipyridine (bpy)) in solution and in cellulose acetate polymer matrix were investigated. The axial ligands substitution was made aiming to evaluate the photophysical properties and the solubility in different solvents. Therefore, dissimilar from the free porphyrin, non-polar solvents (as toluene) favours the quantum yield of iridium(III)porphyrins and ligands with a more extended π-conjugated compound as bpy results in higher yields. Moreover, despite all the porphyrins reveals a negative solvatochromism, the substitution of Cl(CO) ligand by bpy ligand exhibits similar solubility either on non-polar or polar solvents. The observed photoluminescence (PL) at room temperature appears at NIR region in contrast to the previously reported iridium(III) porphyrins. Comparing with free porphyrin H2TTP, the red/NIR PL spectra of the iridium(III)porphyrins (either in solution and in the polymer matrix) reveals remarkable changes. Particularly, a more significative decrease of the red/NIR intensity ratio was detected for [Ir(ttp)(bpy)2] 2 where the maxima of the NIR emission can be adjusted under suitable excitation wavelength." @default.
• W3014320178 created "2020-04-10" @default.
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• W3014320178 date "2020-07-01" @default.
• W3014320178 modified "2023-10-01" @default.
• W3014320178 title "Iridium(III)porphyrin arrays with tuneable photophysical properties" @default.
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• W3014320178 doi "https://doi.org/10.1016/j.saa.2020.118309" @default.
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