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• W3015133799 abstract "In this study, we report independent measurements of all stable isotope ratios of gadolinium. Our study employs multicollector inductively coupled plasma mass spectrometry (MC-ICPMS) with National Research Council Canada (NRC) HALF-1 isotopic hafnium standard as a primary calibrator and surveys four commercial gadolinium materials, including a NRC candidate isotopic reference material, GADS-1. The isotopic composition of gadolinium is determined using the regression model without reliance on conventional normalizing isotope ratios or mass-dependent isotope ratio correction models. In this work, all gadolinium isotope ratios were obtained from 160Gd/158Gd which, in turn, was measured from hafnium 178Hf/177Hf either directly or indirectly through 167Er/166Er. The latter approach was used for the final determination of gadolinium isotopic composition, as it provides smaller combined uncertainty. We report high-precision measurements of the isotopic composition of gadolinium, which support a revised standard atomic weight. Isotope amount ratios of R152/158 = 0.008 20(2)k=1, R154/158 = 0.087 98(12)k=1, R155/158 = 0.596 81(63)k=1, R156/158 = 0.825 08(57)k=1, R157/158 = 0.630 60(22)k=1, and R160/158 = 0.879 10(60)k=1, and the atomic weight of Ar(Gd) = 157.2502(6)k=1 were obtained for gadolinium in GADS-1." @default.
• W3015133799 created "2020-04-10" @default.
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• W3015133799 date "2020-04-08" @default.
• W3015133799 modified "2023-09-25" @default.
• W3015133799 title "Determination of the Isotopic Composition of Gadolinium Using Multicollector Inductively Coupled Plasma Mass Spectrometry" @default.
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• W3015133799 doi "https://doi.org/10.1021/acs.analchem.0c00531" @default.
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• W3015133799 hasPublicationYear "2020" @default.
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