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- W3015266502 abstract "Smooth basal surfaces of illite were prepared successfully, and the interaction forces between a Si₃N₄ tip and illite basal surface with various concentrations of divalent cations in 10 mM KCl solution at pH 8.0 and 10.8 were measured using an atomic force microscope (AFM). The influence of divalent cation concentration on the interaction forces was investigated, and the surface potentials of the basal surfaces in varying concentrations of divalent cation solutions were determined by fitting the interaction forces with the classical Derjaguin–Landau–Verwey–Overbeek (DLVO) theory. With an increasing Caᴵᴵ or Mgᴵᴵ concentration, the surface potentials became less negative in pH 8.0 solution, while the surface potentials reversed from negative to positive after addition of 1.0 mM or more divalent cations in pH 10.8 solution. Electrostatic interaction and specific adsorption were the major contributors to the interaction between divalent cations and illite basal surface in solutions at pH 8.0 and 10.8, respectively. Caᴵᴵ and Mgᴵᴵ cations had a similar effect magnitude on the illite basal surfaces at pH 8.0. In contrast, Mgᴵᴵ cations had a more profound effect than Caᴵᴵ on the surface potential of the illite basal surface in pH 10.8 solution, likely due to the low solubility of Mg(OH)₂ at this pH. This quantitative description of the illite basal surface charge influenced by divalent cations can provide fundamental insight into the mechanisms of tailings treatment and slime coatings in minerals processing." @default.
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- W3015266502 date "2019-01-01" @default.
- W3015266502 modified "2023-09-27" @default.
- W3015266502 title "Probing Interaction of Divalent Cations with Illite Basal Surfaces by Atomic Force Microscopy" @default.
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