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- W3016690739 abstract "Abstract Controllable wetting state on nanotextured surfaces is of fundamental importance in diverse applications, including self-cleaning, droplet manipulation, and lubrication. The Cassie–Baxter (CB) state, which has attracted broad interests due to the dramatic reduction of solid/liquid contact, can easily break down and the inverse transition (dewetting) is highly challenging. Herein, via molecular dynamics simulation, we show that the regulation of geometrical parameters characterizing the graphene-based surfaces enables one to control the wetting states. Our results demonstrate that decoration of carbon nanopillars on graphene could favor dewetting transition as solid surface fraction increases to a critical value. Furthermore, the ability repelling water for solid surface is highly sensitive to the local density distribution of water droplet along the direction perpendicular to nanopillared graphene. Importantly, the mechanistic pathway of self-recovery of CB state is illustrated in details. Dewetting initiates with the vapor cavity nucleation at the basal surface associated with the bottom water-graphene adhesion force, then the ascend of droplet exhibits strong dependence on the subsequent spontaneous expand of vapor cavity which is necessary to achieve the dewetting transition. Our results provide a rational way to achieve dewetting process, which could guide further design of engineering devices with controllable wetting-related applications." @default.
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- W3016690739 date "2020-08-01" @default.
- W3016690739 modified "2023-10-12" @default.
- W3016690739 title "Controllable dewetting transition on graphene-based nanotextured surfaces" @default.
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- W3016690739 doi "https://doi.org/10.1016/j.apsusc.2020.146374" @default.
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