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- W3017092710 abstract "Abstract To design novel conjugated polymers and improve interfacial interaction with semiconductor is one of directions to develop high-efficient photocatalysts with harvesting photons and boosting catalytic activities. Herein, two novel linear conjugated polymers poly[(thiophene-ethylene-thiophene)-thiophene] (PTET-T) and poly[(thiophene-ethylene-thiophene)-thiophene-3-carboxylic acid] (PTET-T-COOH) were successfully synthesized by a simple Stille coupling reaction. Their heterojunction with TiO 2 , i.e, PTET-T/TiO 2 (C1) and PTET-T-COOH/TiO 2 (C2), exhibited outstanding photocatalytic activity for degrading Rhodamine B, methylene blue and tetracycline. The energetic “lock-in effect” between PTET-T-COOH and TiO 2 through carboxyl groups and hydroxyl groups interaction has been proved to greatly improve the interface charge transfer ability and suppress the electron-hole recombination in PTET-T-COOH/TiO 2 . Thus, by regulating the dosage of polymers, the 15% PTET-T-COOH/TiO 2 showed the optimized photocatalytic activity with excellent chemical stability, and its kinetic rate constant was determined to be 41.7 times of that of TiO 2 . This work provided a new effective strategy of designed and explored organic semiconductor-inorganic heterojunction photocatalysts with broaden absorption, repeatability and high-charge mobility." @default.
- W3017092710 created "2020-04-24" @default.
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- W3017092710 date "2020-04-16" @default.
- W3017092710 modified "2023-10-16" @default.
- W3017092710 title "A novel Strategy of Lock-in Effect between Conjugated Polymer and TiO2 towards Dramatic Enhancement of Photocatalytic Activity under Visible Light" @default.
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- W3017092710 doi "https://doi.org/10.1038/s41598-020-63623-2" @default.
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