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• W3017368936 abstract "There is a critical need for sustainable routes to produce hydrogen peroxide, H2O2. A promising approach involves direct synthesis from molecular hydrogen and oxygen at (sub)ambient temperatures using unmodified supported Pd catalysts, which are limited by low selectivities. Controlling the environment of Pd active sites via surface ligands is shown to enhance selectivity. Trends among a myriad of surface ligands (i.e., phosphines, thiols, weakly bound molecules) suggest that those containing H-bonding groups lead to the highest H2O2 production, potentially by affecting reaction energetics via H-bonding with key intermediates. These insights lay the groundwork for ligand design to achieve the optimal catalyst performance for H2O2 synthesis." @default.
• W3017368936 created "2020-04-24" @default.
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• W3017368936 date "2020-04-13" @default.
• W3017368936 modified "2023-10-16" @default.
• W3017368936 title "Tunable Catalytic Performance of Palladium Nanoparticles for H₂O₂ Direct Synthesis via Surface-Bound Ligands" @default.
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• W3017368936 doi "https://doi.org/10.1021/acscatal.0c01517" @default.
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