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- W3017619093 abstract "We show that the lifetime of ultracold ground-state Rb87Cs133 molecules in an optical trap is limited by fast optical excitation of long-lived two-body collision complexes. We partially suppress this loss mechanism by applying square-wave modulation to the trap intensity, such that the molecules spend 75% of each modulation cycle in the dark. By varying the modulation frequency, we show that the lifetime of the collision complex is 0.53±0.06 ms in the dark. We find that the rate of optical excitation of the collision complex is 3−2+4×103 W−1 cm2 s−1 for λ=1550 nm, leading to a lifetime of <100 ns for typical trap intensities. These results explain the two-body loss observed in experiments on nonreactive bialkali molecules.Received 7 February 2020Accepted 27 March 2020DOI:https://doi.org/10.1103/PhysRevLett.124.163402Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCold and ultracold moleculesCooling & trappingUltracold collisionsAtomic, Molecular & Optical" @default.
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- W3017619093 date "2020-04-23" @default.
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- W3017619093 title "Loss of Ultracold <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mmultiscripts><mml:mrow><mml:mi>Rb</mml:mi></mml:mrow><mml:mprescripts /><mml:none /><mml:mrow><mml:mn>87</mml:mn></mml:mrow></mml:mmultiscripts><mml:mmultiscripts><mml:mrow><mml:mi>Cs</mml:mi></mml:mrow><mml:mprescripts /><mml:none /><mml:mrow><mml:mn>133</mml:mn></mml:mrow></mml:mmultiscripts></mml:mrow></mml:math> Molecules via Optical Excitation of Long-Lived Two-Body Collision …" @default.
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- W3017619093 doi "https://doi.org/10.1103/physrevlett.124.163402" @default.
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