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• W3017885767 abstract "Sulfones and sulfonamides with an α-CH bond can be easily alkylated by aliphatic alcohols to add the carbon skeleton of the alcohol via a one-step, Ru(II)-catalyzed redox neutral reaction. The reaction requires a substoichiometric amount of base and produces only water as a byproduct. Several pharmaceutically relevant functional groups such as piperidine, morpholine, etc. are well-tolerated under the reaction conditions to give higher value-added products in one step from widely available substrates. The reaction proceeds through a sulfone carbanion addition to an in-situ-generated aldehyde formed via catalytic dehydrogenation and subsequent catalyst-mediated replacement of the secondary alcohol by hydrogen." @default.
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• W3017885767 date "2020-04-20" @default.
• W3017885767 modified "2023-09-27" @default.
• W3017885767 title "Catalytic Sulfone Upgrading Reaction with Alcohols via Ru(II)" @default.
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• W3017885767 doi "https://doi.org/10.1021/acscatal.0c00206" @default.
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