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- W3018450544 abstract "Intermolecular interaction and molecular configuration are of great importance to the formation of liquid crystals (LCs). In this study, we have designed a fluorinated regulator at the end of LC molecules to investigate mesomorphic properties. Dissecting the terminal fluorinated regulator shows 4-fluoro substituent with a polar effect could promote dipole-dipole interaction, 2,6-difluoro substituent with a twist effect could facilitate steric molecular configuration, while 3,5-difluoro substituent with twist & polar effects could regulate not only molecular configuration and π-π interaction but also dipole-dipole interaction. From the independent and joint effects of the three regulating positions, it is concluded that intermolecular interactions (i.e., dipole-dipole interaction, π-π interaction and perfluoroarene-arene interaction) and molecular configuration can be effectively fine-tuned by the degree and pattern of fluorination. In addition, their thermal stabilities are evaluated systematically. These results will provide a further insight into LC molecule design." @default.
- W3018450544 created "2020-05-01" @default.
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- W3018450544 date "2020-07-01" @default.
- W3018450544 modified "2023-10-09" @default.
- W3018450544 title "Dissecting terminal fluorinated regulator of liquid crystals for fine-tuning intermolecular interaction and molecular configuration" @default.
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- W3018450544 doi "https://doi.org/10.1016/j.molliq.2020.113225" @default.
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