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• W3019933517 abstract "The preparation, assembly and dynamic properties of photoswitchable bisphosphine ligands based on the stiff-stilbene scaffold are reported. Directional bonding and coordination-induced assembly allow complexation of these ligands with palladium(II), resulting in the formation of discrete metallo-supramolecular entities. While the Z isomer forms a simple bidentate metallo-macrocycle, an intricate double helicate figure-of-eight dimer is observed with the E ligand. Topologically 3D complexes can thus be obtained from 2D ligands. Upon irradiation with UV light, isomerization of the ligands allows control of the architecture of the formed complexes, resulting in a light-triggered modulation of the supramolecular topology. Furthermore, a mechanistic investigation unveiled the dynamic nature of the helicate chirality, where a transmission of motion from the palladium centers yields an „eight-to-eight“ inversion." @default.
• W3019933517 created "2020-05-01" @default.
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• W3019933517 date "2020-06-03" @default.
• W3019933517 modified "2023-10-17" @default.
• W3019933517 title "Modulation of a Supramolecular Figure‐of‐Eight Strip Based on a Photoswitchable Stiff‐Stilbene" @default.
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• W3019933517 doi "https://doi.org/10.1002/chem.202002051" @default.
• W3019933517 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7384132" @default.
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• W3019933517 hasPublicationYear "2020" @default.
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