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- W3019969059 abstract "Surface induced order–disorder phase transition has been widely studied on flat bulk surfaces, while such a transition is poorly understood on curved surfaces in nanoscale. Here, we report a direct observation of the dynamic behaviors of surface-initiated disordering in Ag₂S nanoparticles using atomic resolution in situ transmission electron microscopy. It was found that the disordering behavior is different from the traditional model that the disordered layer follows a logarithmic thickness dependence with temperature. In particular, the disordering is largely enhanced at higher temperature when the radius of the residual order phase is getting smaller. Moreover, the correlation length of disordered phase was found to be several times larger than the typical value for bulk surfaces. This significantly enhanced disordering in nanoparticles could be attributed to the extra driving force provided by the decreasing of order–disorder interface area." @default.
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- W3019969059 date "2018-01-01" @default.
- W3019969059 modified "2023-09-27" @default.
- W3019969059 title "Direct Observation of Curved Surface Enhanced Disordering in Ag₂S Nanoparticles" @default.
- W3019969059 hasPublicationYear "2018" @default.
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