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- W3020506247 abstract "A series of Ni-Ca-HMS catalysts were prepared by one-step co-assembly synthesis and applied to dry reforming of methane. The promoting effect of CaO on the inhibition of carbon deposition was investigated via the DRM reaction over the Ni-HMS catalysts. The results indicated that the doping of Ca not only significantly enhanced the metal-support interaction, but also decreased the graphitic degree of deposited carbon. Moreover, it was found that the coking-resistance was obviously increased after introducing calcium. The presence of CaO promoted CO2 adsorption and accelerated the removal of carbon. Interestingly, the Ni/Ca ratio also played a vital role. The Ni-Ca-HMS catalyst with Ni/Ca ratio of 3:2 exhibited the highest stability and coke-resistance during continuously reacting in the thermodynamic active zone of coke formation (557 ~ 700 °C). Only 4.2% deposited carbon was produced for 3Ni2Ca-HMS catalyst after dynamically reacting at 650 °C for 48 h, which was much lower than Ni-HMS catalyst (31.7%). Besides, excellent anti-sintering property was also obtained on 3Ni2Ca-HMS catalyst only with the increment of Ni particle size from 3.73 to 3.99 nm." @default.
- W3020506247 created "2020-05-01" @default.
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- W3020506247 date "2020-08-01" @default.
- W3020506247 modified "2023-10-18" @default.
- W3020506247 title "Insight into the role of CaO in coke-resistant over Ni-HMS catalysts for CO2 reforming of methane" @default.
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- W3020506247 doi "https://doi.org/10.1016/j.apsusc.2020.146395" @default.
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