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- W3021090696 abstract "Cu-Fe catalysts prepared from layered double hydroxide (LDH) precursors were applied for the straightforward N-alkylation of aniline with benzyl alcohol in base- and oxidant-free conditions. Among the bimetallic Cu-M catalysts prepared from LDH precursors, the Cu-Fe catalyst showed the most active catalysis for the direct N-alkylation of aniline with benzyl alcohol to produce 12 % benzylideneaniline and 88 % N-benzylaniline. Synergistic catalysis between the Cu and Fe species in the Cu-Fe catalyst is crucial for the catalytic cycle of the N-alkylation. In the mechanistic studies reported here, the hydrogen-borrowing approach was intensely observed using in situ fourier-transform infrared spectroscopy (FT-IR) measurements and reaction sequence studies." @default.
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- W3021090696 date "2020-07-01" @default.
- W3021090696 modified "2023-10-11" @default.
- W3021090696 title "One-pot synthesis of aniline N-alkylation from benzyl alcohol over Cu-Fe catalyst" @default.
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- W3021090696 doi "https://doi.org/10.1016/j.apcata.2020.117519" @default.
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