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- W3021342364 abstract "Phenyl-perfluorophenyl polar-π interactions have been revisited for the design and fabrication of functional supramolecular systems. The relatively weak associative interactions (ΔG ≈ -1.0 kcal/mol) have limited their use in aqueous self-assembly to date. Herein, we propose a strategy to strengthen phenyl-perfluorophenyl polar-π interactions by encapsulation within a synthetic host, thus increasing the binding affinity to ΔG= -15.5 kcal/mol upon formation of heteroternary complexes through social self-sorting. These heteroternary complexes were used as dynamic, yet strong, cross-linkers in the fabrication of supramolecular gels, which exhibited excellent viscoelasticity, stretchability, self-recovery, self-healing, and energy dissipation. This work unveils a general approach to exploit host-enhanced polar-π interactions in the design of robust aqueous supramolecular systems." @default.
- W3021342364 created "2020-05-13" @default.
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- W3021342364 date "2020-04-13" @default.
- W3021342364 modified "2023-09-23" @default.
- W3021342364 title "Host-Enhanced Phenyl-Perfluorophenyl Polar-π Interactions." @default.
- W3021342364 doi "https://doi.org/10.17863/cam.52180" @default.
- W3021342364 hasPublicationYear "2020" @default.
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