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- W3021563181 abstract "Single-atom catalysts have demonstrated their superiority over other types of catalysts for various reactions. However, the reported nitrogen reduction reaction single-atom electrocatalysts for the nitrogen reduction reaction exclusively utilize metal-nitrogen or metal-carbon coordination configurations as catalytic active sites. Here, we report a Fe single-atom electrocatalyst supported on low-cost, nitrogen-free lignocellulose-derived carbon. The extended X-ray absorption fine structure spectra confirm that Fe atoms are anchored to the support via the Fe-(O-C2 )4 coordination configuration. Density functional theory calculations identify Fe-(O-C2 )4 as the active site for the nitrogen reduction reaction. An electrode consisting of the electrocatalyst loaded on carbon cloth can afford a NH3 yield rate and faradaic efficiency of 32.1 μg h-1 mgcat.-1 (5350 μg h-1 mgFe-1 ) and 29.3 %, respectively. An exceptional NH3 yield rate of 307.7 μg h-1 mgcat.-1 (51 283 μg h-1 mgFe-1 ) with a near record faradaic efficiency of 51.0 % can be achieved with the electrocatalyst immobilized on a glassy carbon electrode." @default.
- W3021563181 created "2020-05-13" @default.
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- W3021563181 date "2020-05-27" @default.
- W3021563181 modified "2023-10-16" @default.
- W3021563181 title "Electrocatalytically Active Fe‐(O‐C<sub>2</sub>)<sub>4</sub>Single‐Atom Sites for Efficient Reduction of Nitrogen to Ammonia" @default.
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- W3021563181 doi "https://doi.org/10.1002/anie.202005930" @default.
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