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- W3021737314 endingPage "2572" @default.
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- W3021737314 abstract "For decades, the formal metal addenda substitution in the matrix of bulk metal oxides has been a prolific strategy to develop numerous (non‐)stoichiometric all‐inorganic compounds with tunable electronic and magnetic properties, and broad technological applications. In contrast to bulk mixed‐metal oxides, the formal metal‐addenda substitution in their molecular equivalents typically leads to stoichiometrically precise mixed‐metal cluster formulations which retain the overall structural topology of the monometallic archetype, but exhibit pronounced differences in terms of reactivity and spectroscopic properties. These mixed‐metal molecular metal oxides often show complex configurational isomerism that has been the subject of many experimental and theoretical studies. The mixed‐addenda metal‐oxo clusters are most prominent among the classical plenary (that contain no vacant metal sites) polyoxometalate (POMs) archetypes, which have emerging applications in homogeneous catalysis and material science (e.g. formation of open frameworks), and have also been explored in heterogeneous metal organic framework (MOF) catalysts. Therefore, this article provides comprehensive theoretical and experimental insights into the isomer problem of mixed‐addenda molecular metal oxides and their applications." @default.
- W3021737314 created "2020-05-13" @default.
- W3021737314 creator A5030890226 @default.
- W3021737314 creator A5032807322 @default.
- W3021737314 creator A5049709560 @default.
- W3021737314 date "2020-05-27" @default.
- W3021737314 modified "2023-10-11" @default.
- W3021737314 title "Metal‐Addenda Substitution in Plenary Polyoxometalates and in Their Modular Transition Metal Analogues" @default.
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