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• W3021739616 abstract "Lead halide perovskite has emerged as a promising photovoltaic material due to its excellent power conversion efficiency (PCE). However, the toxicity problem of lead-based perovskite hampers the commercialization of perovskite solar cells. Here, we develop several Sb(V) complexes with pyridyl cations and serve as absorber layer for lead-free perovskite solar cells. The designed complexes were based on 4-tert-butylpyridine (tBP) and N-ethylpyridinium (N-EtPy) cations with bandgaps of 2.01 eV and 1.95 eV, which showed their potential for solar cells and optoelectronic applications. We also found a chemical rule for stable Sb complexes in terms of the bond connectivity of pnictogen-antimony. Initial studies produce a solar cell with a PCE of 0.9% and offer inspiration for further exploration of environment-friendly perovskite families. Sb(V) complexes with pyridyl cations were synthesized and served as absorber layer for lead-free perovskite solar cells. The Sb-based solar cell produced a PCE of 0.9% and offered inspiration for further exploration of environment-friendly perovskite families." @default.
• W3021739616 created "2020-05-13" @default.
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• W3021739616 date "2020-08-05" @default.
• W3021739616 modified "2023-09-25" @default.
• W3021739616 title "Synthesis of Sb(V) Complexes with Pyridyl Cations and Application for Lead-free Perovskite Solar Cells" @default.
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• W3021739616 doi "https://doi.org/10.1246/cl.200208" @default.
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